LINQ transform Dictionary to Dictionary

Use ToDictionary ?

orignalDictionary.ToDictionary(kp => kp.Value, kp => kp.Key);

This works because IDictionary<TKey,TElement>; is also an IEnumerable<KeyValuePair<TKey,TElement>>;. Just be aware that if you have duplicate values, you will get an exception.

In case you have duplicate values, you will need to decide on what to do with them. One simple way would be to ignore duplicates by grouping on Value first, then make the dictionary.

originalDictionary
.ToLookup(kp => kp.Value)
.ToDictionary(g => g.Key, g => g.First().Key);