Get all column names of a DataTable into string array using (LINQ/Predicate)

Try this (LINQ method syntax):

string[] columnNames = dt.Columns.Cast<DataColumn>()
                                 .Select(x => x.ColumnName)
                                 .ToArray();  

or in LINQ Query syntax:

string[] columnNames = (from dc in dt.Columns.Cast<DataColumn>()
                        select dc.ColumnName).ToArray();

Cast is required, because Columns is of type DataColumnCollection which is a IEnumerable, not IEnumerable<DataColumn>. The other parts should be obvious.