How to bind to model with Angular Material ?

MatButtonToggle component doesn’t implement ControlValueAccessor therefore you can’t use ngModel on it. ngDefaultControl was introduced for other purposes.

MatButtonToggle is supposed to be a part of mat-button-toggle-group. But if you want to use it as a standalone component and bind model to it here is some example of how you can do it:

<mat-button-toggle 
  [checked]="myFlagForButtonToggle" 
  (change)="myFlagForButtonToggle = $event.source.checked">
    Toggle me!
</mat-button-toggle>

Plunker Example